Manipulating magnetism and transport properties of EuCd2P2 with a low carrier concentration

Abstract

Materials that exhibit strongly coupled magnetic order and electronic properties are crucial for both fundamental research and technological applications. However, finding a material that not only shows remarkable magnetoresistive responses but also has an easily tunable ground state remains a challenge. Here, we report successful manipulation of the magnetic and transport properties of EuCd2P2, which is transformed from an A-type antiferromagnet (TN = 11 K) exhibiting colossal magnetoresistance into a ferromagnet (TC = 47 K) with metallic behavior. The dramatic alteration results from a low hole concentration of 1019 cm-3 induced by changing the growth conditions. Electronic structure and total energy calculations confirm the tunability of magnetism with a small carrier concentration for EuCd2P2. It is feasible to switch between the magnetic states by using field-effect to control the carrier density, thereby changing the magneto-electronic response. The controllable magnetism and electrical transport of EuCd2P2 make it a potential candidate for spintronics.

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