Nonmagnetic Phase Transition in La3TiSb5 Observed in 121Sb Nuclear Quadrupole Resonance

Abstract

We measured the electrical resistivity and the 121Sb nuclear quadrupole resonance (NQR) spectra of La3TiSb5, which is a nonmagnetic reference system for a locally noncentrosymmetric antiferromagnet Ce3TiSb5, in order to determine its physical properties. The resistivity exhibited a hump anomaly at 120 K, suggesting a phase transition. The NQR spectra split below 110 K, whereas the nuclear spin-lattice relaxation exhibited no anomalies. These results can be explained by the incommensurate charge-density-wave (CDW) transition. This finding suggests the importance of quasi-one-dimensional characteristics and CDW instability in these systems.

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