Anomalous Lasing Behavior in a Nonlinear Plasmonic Random Laser

Abstract

An unprecedented double-threshold lasing behavior has been observed in a plasmonic random laser composed of Au nanoislands decorated on vertically standing ZnO nanorods, infiltrated with dye-doped polymer matrix. The strong coupling of random laser modes to plasmonic nanocavities results in a dominant absorption of the random laser emission, leading to the first unusual lasing threshold. At higher pump fluences, the nonlinear optical behavior of the Au nanoislands induces a second lasing threshold. Various statistical tools have been employed to analyze the intensity fluctuations of the random laser modes, validating this unique lasing behavior.