Topological Charge Quadrupole Protected by Spin-Orbit U(1) Quasi-Symmetry in Antiferromagnet NdBiPt

Abstract

The interplay of symmetry and topology in crystal solids has given rise to various elementary excitations as quasiparticles. Among these, those with significant Berry-phase-related transport responses are of particular interest. Here, we predict a new type of quasiparticle called topological charge quadruple (TCQ), which is analogous to a charge quadrupole but consists of two closely-packed pairs of Weyl points in momentum space, specifically in a half-Heusler antiferromagnet NdBiPt. Interestingly, the TCQ is protected by the spin-orbit $U(1)$ quasi-symmetry, rather than any exact crystallographic symmetries. This quasi-symmetry restricts the energy splitting induced by symmetry-lowering perturbations to a second-order effect. Furthermore, the closely located Berry curvature sources and sinks in the TCQ lead to a large Berry curvature dipole, resulting in a significant nonlinear Hall effect. Our work opens an avenue for designing novel quasiparticles using quasi-symmetries and developing materials with enhanced nonlinear responses.