Two-dimensional spectroscopy of open quantum systems
Abstract
Two-dimensional spectroscopy is discussed for open quantum systems with multiple simultaneously measurable fluxes. In particular, we discuss a junction where optical measurements of photon flux are complemented with simultaneous transport measurements of electron currents. Theory of two-dimensional spectroscopy in both fluxes is developed employing non-self-consistent nonequilibrium Green's function formulation. Theoretical derivations are illustrated with numerical simulations within generic junction model.
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