Opposite-Mirror-Parity Scattering as the Origin of Superconductivity in Strained Bilayer Nickelates

Abstract

We study the electronic structure and doping-dependent instabilities of strained La3Ni2O7 thin films using first-principles and functional renormalization group methods. We demonstrate that ordering tendencies are governed by Fermi surface scattering between electrons of opposite mirror parity. Under moderate hole doping, when the dz2 bonding band becomes incipient or crosses the Fermi level, robust s-wave superconductivity emerges from cooperative interlayer pairing reinforced by two competing spin-density-wave fluctuations. Compressive strain favors superconductivity in NiO2 bilayers slightly away from the interface, whereas tensile strain induces pair-breaking nesting that suppresses pairing. Our results establish a unified microscopic scenario for superconductivity in pressurized bulk and strained thin-film nickelates, providing new insights into high-Tc pairing in correlated quantum materials.

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