Enhanced anomalous Hall effect in the topological Kagome metal Cs(V$_{1-x}$Mn$_x$)$_3$Sb$_5$

Abstract

As a fundamental physical phenomenon, achieving and controlling a large anomalous Hall effect (AHE) is crucial for advancing the understanding of topological physics and for developing applied technologies in spintronics. The recently discovered topological Kagome metal $A$V$_3$Sb$_5$ ($A =$ K, Rb, Cs)exhibits a significant AHE along with charge density wave (CDW) and superconductivity, providing an ideal platform to study the interactions between nontrivial band topology, CDW, and superconductivity. In this study, we systematically investigated the evolution of CDW, superconductivity, and AHE in electron (Mn)-doped Cs(V$_{1-x}$Mn$_x$)$_3$Sb$_5$ single crystals. The experimental results show that electron doping rapidly suppresses superconductivity, while the CDW order remains relatively robust. Meanwhile, a significantly enhanced AHE, with a maximum anomalous Hall conductivity (AHC) of ~25331 \Ohm ^{-1}\cm^{-1} and an anomalous Hall angle of 6.66% occurs at a relatively low doping level of $x = 0.03$. Based on the Tian-Ye-Jin (TYJ) scaling model, such a significant enhancement AHC is mainly dominated by the skew scattering. We speculated enhanced skew scattering between electrons and Mn originating from the strengthened spin-orbital coupling. Our finding provides important guidance for the design and development of transverse transport properties in topological Kagome materials.