Superconducting Spin-Singlet QuBit in a Triangulene Spin Chain

Abstract

Chains of triangular nanographene (triangulene), recently identified as realizing the valence-bond solid phase of a spin-1 chain, offer a promising platform for quantum information processing. We propose a spin-singlet qubit based on these chains grown on a superconducting substrate. Using the numerical renormalization group (NRG), we identify a manifold consisting of the two lowest-lying, spin-singlet states isolated from doublet states of opposite fermion parity, which undergo an avoided crossing. A qubit utilizing these states is thus protected from random Zeeman and/or spin-orbit coupling. Despite the unavoidable effect of quasiparticle poisoning on qubit performance, the isolation of the singlet states offers additional protection. In addition, we introduce a mesoscopic device architecture, based on a triple quantum dot coupled to a superconducting junction, that quantum simulates the spin chain and enables control and readout of the qubit. An effective two-level description of the device is validated using time-dependent NRG.