Light-field dressing of transient photo-excited states above EF

Abstract

Time-periodic light-field provides an emerging pathway for dynamically engineering quantum materials by forming hybrid states between photons and Bloch electrons. So far, experimental progress on light-field dressed states has been mainly focused on the occupied states, however, it is unclear if the transient photo-excited states above the Fermi energy EF can also be dressed, leaving the dynamical interplay between photo-excitation and light-field dressing elusive. Here, we provide direct experimental evidence for light-field dressing of the transient photo-excited surface states above EF, which exhibits distinct dynamics with a delay response as compared to light-field dressed states below EF. Our work reveals the dual roles of the pump pulse in both photo-excitation and light-field dressing, providing a more comprehensive picture with new insights on the light-induced manipulation of transient electronic states.

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