Strong altermagnetism and topological features in a two-dimensional van der Waals heterostructure via broken time reversal symmetry

Abstract

The advent of altermagnetism, a new phase of magnetism, has garnered significant interest due to its extraordinary spin-polarized electronic bands despite zero net magnetization. Such spin-symmetry-guided robust non-relativistic alternating spin splitting in a compensated collinear magnet presents a novel platform for magnetotransport and nontrivial topology. Predominantly, altermagnetic behavior is observed in bulk magnetic materials upon incorporating external perturbations. However, van der Waals heterostructures can offer exceptional flexibility in tailoring their various emerging properties without the need for external perturbations in the two-dimensional regime. Here, an unconventional time reversal symmetry breaking with sizeable spin splitting via broken space-spin symmetry (\textit{P$\mathcal{T}$}) has been demonstrated in an antiferromagnet/nonmagnet vdW heterostructure. The lifted Kramer's degeneracy alongwith spin-orbit interactions result in non-zero Berry curvature, contributing to the outstanding magnetotransport with a large value of anomalous Hall conductivity ($\sim 732.9\ {\mathit{\Omega}}^{-1}{cm}^{-1}$). The presence of relativistic spin-orbit interactions in addition to predominant non-relativistic effects governed spin-momentum locking with a weak out-of-plane Dzyaloshinskii-Moriya interaction, which induces small spin canting. Further, the lowest magnetic anisotropy energy confirms collinear antiferromagnetic ground state. In particular, a nontrivial topology is observed along the surface [001], which is confirmed by the non-zero Chern number. This study provides a novel approach to realize strong altermagnetism in broken space-spin symmetry systems and fosters emergent transport behaviors.