Evaluation of bound-state β--decay half-lives of fully ionized atoms
Abstract
Bound-state β--decay is a rare radioactive process where the created electron is trapped in an atomic orbital instead of being emitted. It can be observed in highly ionized atoms in particular when normal beta decay is energetically forbidden, but bound-state decay is still possible. In this work we present a systematic theoretical study on the bound-state β--decay of fully ionized atoms where key nuclear inputs include the nuclear matrix elements (expressed through ft values) and the lepton phase-space volume function. We present a method to evaluate nuclear matrix elements for fully forbidden β- transitions in neutral atoms, from the inverse electron capture process using the Takahashi-Yokoi model and account for the impact of electron capture to different atomic orbitals on the resulting half-lives. Decay rates for bound-state β--decays of nuclei 163Dy, 193Ir, 194Au, 202Tl, 205Tl, 215At, 222Rn, 243Am, and 246Bk are calculated, where the normal beta decay is forbidden. In addition, we compute the bound-state β- decay rates for nuclei 187Re, 227Ac, and 228Ra, observing enhancements by factors of 102 to 104 relative to their neutral-atom counterparts. Our results show that the half-lives of certain bare nuclei are significantly shorter than those of the corresponding neutral atoms, identifying them as promising candidates for future experimental investigation. The theoretically predicted half-lives of the bound-state β- decay could provide valuable inputs for various astrophysical studies.
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