Plasmon-enhanced quadrupole transitions of Rydberg excitons in Cu2O

Abstract

A mechanism for amplification of weak quadrupole transitions of Rydberg excitons in Cu2O by a plasmonic nanostructure is investigated. The theoretical description of exciton-plasmon interaction is presented and a field averaging approximation is proposed for calculations involving large excitons. Various types of copper, silver and gold-based plasmonic nanostructures are considered and their potential for enhancing quadrupole transitions is evaluated.

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