Displacement-Field-Driven Transition between Superconductivity and Valley Ferromagnetism in Transition Metal Dichalcogenides

Abstract

Recent experiments have observed transitions between superconductivity and correlated magnetism in twisted bilayer WSe2 near van-Hove fillings, driven by the displacement field D. Motivated by the experiment, we theoretically propose a general mechanism for a D-controlled transition between superconductivity and ferromagnetism in two-dimensional (2D) spin-orbit-coupled hexagonal systems, where van Hove singularities (VHS) lie on the Fermi level. We show that such a transition can be naturally captured by a simple VHS-only model without Fermi surface details, where the inter-VHS interactions that govern the Fermi surface instabilities is controlled by D through the band projection of screened Coulomb interaction. By treating this simple model with renormalization group technique beyond mean-field level, we find that a chiral d/p-wave superconductivity naturally dominates under a weak displacement field D<Dc. At a stronger displacement field D>Dc, a valley ferromagnetic phase (vFM) takes over, which is spatially non-uniform due to valley-modulated magnetization. Finally, we discuss generic conditions for the predicted superconductivity-to-ferromagnetism transition to take place in the rich family of few-layer hexagonal van der Waals material systems. Taking twisted bilayer WSe2 as a case study, we discuss experimental detections that can falsify our prediction.

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