Tunable Two-Dimensional Electron Gas at the Interfaces of Ferroelectric Potassium Tantalate Niobates

Abstract

The heterointerfaces at complex oxides have emerged as a promising platform for discovering novel physical phenomena and advancing integrated sensing, storage, and computing technologies. Nevertheless, achieving precise control over a two-dimensional electron gas (2DEG) in a ferroelectric oxide-based field-effect transistor (FET) configuration remains challenging. Here, we firstly demonstrate a tunable 2DEG system fabricated by depositing an amorphous LaAlO3(LAO) film onto a (001)-oriented ferroelectric potassium tantalate niobate substrate. Interfaces grown under high-temperature and high-oxygen-pressure conditions exhibit a good metallic conduction. Notably, well-defined metallic 2DEGs displaying pronounced hysteresis and persistent electric-field-modulated resistance are observed below 108 K, achieving a resistance modulation of 11.6% at 7 K. These results underscore the potential for extending such behavior to other oxide-based 2DEG systems and facilitate further exploration of ferroelectric metals in complex oxide heterostructures.