Orbital Separation of Charge Order and Superconductivity in La2-xSrxCuO4

Abstract

We report a combined x-ray absorption (XAS) and oxygen K-edge resonant inelastic x-ray scattering (RIXS) study of charge order in underdoped La2-xSrxCuO4 (x=0.125) under uniaxial c-axis pressure. We find that compressive c-axis strain modifies the charge order only within the superconducting state, with a striking polarization dependence: suppression in the dx2-y2 channel and enhancement in the dz2 channel. X-ray absorption spectra reveal concomitant strain-induced modifications of the oxygen pre-edge and upper Hubbard band, consistent with increased dz2 orbital admixture. Our results suggest that c-axis pressure drives an orbital separation between superconductivity, rooted in dx2-y2 states, and charge order, which gradually shifts to the dz2 channel. This orbital separation reveals a way for superconductivity and charge order to coexist in the cuprates with minimal competition. Furthermore, it suggests that the multi-order phase diagram of La2-xSrxCuO4 cannot be realistically described within single band models usually used to describe cuprate physics.

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