Spin-dependent Raman and Brillouin light scattering on excitons in CsPbBr3 perovskite crystals
Abstract
The spin properties of excitons and charge carriers in CsPbBr3 lead halide perovskite crystals are investigated by spin-dependent light scattering in magnetic fields up to 10 T. Spin-flip Raman scattering spectra measured under resonant excitation of exciton-polaritons show a rich variety of features provided by the Zeeman splittings of excitons and of electrons and holes interacting with the excitons. The magnitudes and anisotropies of their Land\'e g-factors are measured. A detailed consideration of the responsible mechanisms is presented and discussed in relation to the experimental data, in particular on the polarization properties of the Raman spectra. We consider several mechanisms for the combined spin-flip Raman scattering processes involving resident carriers and photoexcited excitons and suggest new ones, involving trions in the intermediate scattering state. A double electron spin-flip caused by the exciton interaction with two localized or donor-bound electrons is revealed. The spectral lines of Brillouin light scattering on exciton-polaritons shift in energy and become polarization-sensitive in magnetic field, evidencing the splitting of the exciton-polariton dispersion.
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