Probing multipolar order in the candidate altermagnet MnF$_2$ through the elastocaloric effect under strain

Abstract

Altermagnets break a combination of time-reversal and rotational symmetries without generating a net magnetization. As such, the order parameter of $d$-wave altermagnets has the same symmetry as magnetic multipoles, and couples to the product of a magnetic field and uniaxial strain. We combine elastocaloric experiments, free-energy modeling, and first-principles calculations on MnF$_2$ to establish a thermodynamic probe of the predicted finite-temperature altermagnetic critical point. These results pave the way to explore altermagnetic quantum criticality in $d$-wave materials and beyond.