Enhanced Yield Rate of 229mTh via Cascade Decay in Storage Rings and Electron Beam Ion Traps

Abstract

The low-energy nuclear isomeric state of 229mTh provides a unique bridge between nuclear and atomic physics, enabling applications such as nuclear clocks and precision metrology. However, efficient and controllable production of 229mTh remains a major experimental challenge. We propose an efficient scheme to produce the 229mTh in storage rings (SRs) and electron beam ion traps (EBITs), using a cascade decay pathway. Highly charged ions are excited to higher nuclear states via nuclear excitation by inelastic electron scattering (NEIES) and nuclear excitation by electron capture (NEEC), followed by radiative or internal conversion cascades that populate the isomer. Our calculations demonstrate that, under typical SRs and EBITs conditions, optimized indirect excitation pathways significantly enhance 229mTh production rate. In particular, NEIES can provide an enhancement of up to four orders of magnitude through cascade de-excitation at high energies, while NEEC can contribute an additional enhancement of up to several tens of times. Such a significant increase in the 229mTh yield rate would facilitate its application in various nuclear photonics fields, especially in the development of atomic nuclear clocks.

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