Sign control of photocurrents by spin-group-symmetry breaking in altermagnetic insulators

Abstract

Controlling physical responses through symmetry breaking is a central paradigm in quantum materials, enabling novel functionalities. Here we determine the effects of spin-group-symmetry breaking on nonlinear optical responses of collinear altermagnetic insulators. Using shear strain as an example, we show that the direction of symmetry-breaking induced components of charge and spin photocurrents are locked to the sign of the strain. In the absence of spin-orbit coupling, this effect is intuitively captured by the spin-gap asymmetry--an imbalance between spin-up and spin-down direct band gaps which couples trilinearly with the N\'eel order and the strain. We demonstrate this mechanism with density functional theory calculations on the recently proposed altermagnet CuWP$_2$S$_6$. Having symmetry-guided control of both charge and spin photocurrents allows, vice versa, to reveal and investigate altermagnetism in insulating materials by exploration of their optical responses.