Interface and Strain Control of Emergent Weyl Semimetallic Phase in SrNbO$_{3}$/LaFeO$_{3}$ Heterostructures

Abstract

Realizing correlated topological semimetallic phases in bulk transition-metal oxides remains challenging due to rigid lattice symmetry, correlation-induced gap opening, and limited structural tunability. However, complex-oxide thin films and heterostructures provide a powerful platform to stabilize topological phases by tailoring the requisite lattice symmetry through strain control and interface design. In this study, we demonstrate the emergence of Weyl-like electronic states and associated chiral transport in SrNbO$_3$ (SNO)/LaFeO$_3$ (LFO) bilayers. Transport measurements reveal signatures consistent with nontrivial topology, including large non-saturating MR, a nonlinear Hall response, and a chiral anomaly like feature in longitudinal magnetotransport under parallel electric and magnetic fields ($\mathbf{B} \parallel \mathbf{I}$). In addition, we observe a \textcolor{black}{signature} of anomalous Hall contribution, likely arising from \textcolor{black}{proximity effect induced by LFO layers at the interface}. First-principles calculations reveal an $a^0a^0c^-$ rotation pattern of the NbO$_6$ octahedra, together with interfacial lattice distortions in the SNO layer that drive the emergence of a twofold degenerate Weyl semimetallic phase protected by screw axis lattice symmetry. This is further confirmed by Berry curvature calculations, which show opposite sign Berry curvature peaks for the upper and lower band characteristic of a Weyl node. Our combined experimental and theoretical results highlight the critical role of strain and interfacial octahedral distortions in stabilizing Weyl phase in transition metal based perovskite bilayer.