Investigating the intrinsic anomalous Hall effect in MnPt3 topological semimetal

Abstract

The cubic Cu3Au-type XPt3 family (X = V, Cr, and Mn) is a topological semimetal characterized by anti-crossing gapped nodal lines near the Fermi level, which give rise to significant Berry curvatures and thus to the anomalous Hall effect (AHE). Among the three members, CrPt3 has been experimentally verified to exhibit a large anomalous Hall conductivity (AHC), while its counterparts MnPt3 and VPt3 remain largely unexplored. Here, a series of MnPt3 thin films with varying thicknesses (20--70 nm) was epitaxially grown on the MgO substrates using magnetron sputtering and was systematically investigated by magnetization, electrical resistivity, and Hall resistivity measurements. MnPt3 films undergo a ferromagnetic transition at a Curie temperature TC, which increases as the film thickness increases, reaching 344 K for the 70-nm-thick film. All the anomalous Hall transport properties of MnPt3 films, including the resistivity, conductivity, and angle, exhibit a strong correlation with their magnetic properties. The scaling analysis suggests that the intrinsic Berry-curvature mechanism dominates the observed AHE, while the extrinsic contributions are much smaller. The intrinsic AHC increases as the film thickness increases, while the extrinsic AHC is thickness-independent. Such an enhanced intrinsic AHC in the MnPt3 films is most likely attributed to the strain effect, implying that it serves as an effective method to tune the electronic band topology in the XPt3 topological semimetal.

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