Programmable dipolar interaction geometry selects stripe-family order in a molecular lattice quantum simulator

Abstract

Microwave-dressed polar molecules offer a route to lattice quantum simulators in which the angular form of long-range dipolar interactions, not only their overall strength, can be engineered. We study this setting in a minimal hard-core Bose lattice model on a square optical lattice, with particles interacting through a sign-changing non-axisymmetric dipolar tail \mathcal V(\mathbf r)\propto (x^2-y^2)/(x^2+y^2)^{5/2} that is repulsive along one lattice axis and attractive along the other. Using worm-algorithm path-integral quantum Monte Carlo simulations, supported by a hard-core spin mapping and a Gutzwiller soft-mode diagnostic, we find two regimes controlled by t/V: at larger t/V the system remains superfluid but develops a pronounced directional stiffness anisotropy, while at smaller t/V it forms a stripe solid selected in the (q,0) axial family, corresponding to real-space stripes parallel to y. The leading ordering wave vector remains in this axial family but reorganizes with filling, showing that the robust ordered object is a family of stripe states rather than one fixed commensurate Bragg peak. Near the closure of the stripe lobe, averaged observables can mimic a narrow supersolid signal; measurement-resolved stripe structure-factor histograms instead reveal first-order switching between superfluid and stripe-solid sectors. NaCs lattice estimates place the relevant V/t window within reach of modest effective dressed dipole moments, linking the predicted stripe-family order and its experimental diagnostics to accessible molecular quantum-simulation scales.