Dynamic nanoscale structural correlations in strontium ruthenate

Abstract

Strontium ruthenate (Sr$_2$RuO$_4$, SRO) has been the subject of intense research as a model quasi-two-dimensional metal with strong electronic correlations and potential exotic multi-component superconductor. Yet the nature of the superconducting state and its emergence remain debated, despite highly detailed knowledge of the normal-state electronic properties. Here we use diffuse neutron and x-ray scattering to uncover self-organized structural fluctuations on the picosecond timescale in SRO. We show that these nanoscale correlations do not originate from extrinsic disorder but rather involve cooperative displacements of oxygen atoms in the quintessential RuO$_2$ planes. Moreover, the observed displacement pattern is consistent with distortions due to incipient orbital order that we obtain in first-principles calculations, which suggests that orbital effects could play a pivotal role in the physics of SRO. Similar dynamic correlations may play a role in the physical properties of a wide range of prominent oxides with closely-related lamellar structures, such as the cuprates and nickelates.