Polarization-Selective Near-Perfect Absorption via Mie-Type Resonance in van der Waals Anisotropic ReS2/α-MoO3/Au Heterostructure

Abstract

We investigate polarization-selective absorption in a visible-wavelength heterostructure consisting of a ReS2 stripe grating, an α-MoO3 spacer, and an Au back-reflector using finite-difference time-domain simulations. For an optimized geometry with a grating period of 500 nm, stripe width of 250 nm, and ReS2 thickness of 80 nm, the structure exhibits near-unity absorption of 99.99\% at 650.5 nm under TE-polarized illumination. The resonant field is concentrated near the outer edges of the ReS2 stripe, while absorption power density is localized in the same region, consistent with a localized edge mode. The absorption response depends strongly on polarization, producing a TE--TM resonance separation of 16.2 nm. Replacing either the biaxial ReS2 layer or the anisotropic α-MoO3 spacer with isotropic equivalents substantially modifies the spectral response and reduces the polarization-dependent wavelength separation. In addition, rotating the crystal orientation of the ReS2/α-MoO3 stack shifts both the resonance wavelength and peak absorption without changing the device geometry. The results show that the combination of anisotropic resonator and spacer layers provides an effective means of controlling resonant absorption and polarization selectivity in van der Waals photonic structures.

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