Thickness-Independent Quantum Geometric Responses Driven by Interlayer Antiferroic Coupling

Abstract

Two-dimensional ferroic materials exhibit rich and intriguing physical phenomena, but their response properties generally depend sensitively on thickness, requiring precise layer-number control and thereby limiting practical applications. Here, we propose a general strategy for realizing thickness-independent quantum geometric responses through symmetry engineering induced by interlayer antiferroic coupling. Using spatial-dependent symmetry analysis, we show that thickness-independent behavior emerges when the symmetry breaking required for a given response is generated by interlayer antiferromagnetic (AFM) or antiferroelectric (AFE) coupling, without invoking topological mechanisms. Our first-principles calculations predict that multilayer MnS in the G-type AFM configuration exhibits a surface-dominated anomalous Hall effect, whose thickness-independent behavior can be significantly influenced by the stacking order. We further propose design principles for achieving thickness-independent anomalous and nonlinear Hall effects driven by interlayer AFE coupling, and suggest potential applications in distinguishing magnetic structures. Our findings open a new route towards robust functional devices based on antiferroic materials.