Diagnosing the origin of quantum oscillation beating in graphene

Abstract

Magnetic quantum oscillations are usually periodic in inverse magnetic field, and their amplitude can show beating when two nearby frequencies interfere. In graphene-based hexagonal systems, such beating can arise from strain-induced pseudomagnetic fields, unequal valley populations, valley-dependent energy shifts, spin-orbit coupling-induced band splitting, or Kekulé distortions. Here, we show that the carrier density and magnetic field dependence of the beating nodes can distinguish these mechanisms. Starting from Onsager's quantization relation, we derive scaling relations for the critical carrier density $N_c$ for the beating nodes as a function of critical magnetic field $B_c$. A pseudomagnetic field gives $N_c\propto B_c^2$, whereas a density-independent valley imbalance gives $N_c\propto B_c$. A constant Dirac-band energy splitting by Zeeman-like spin-orbit coupling also gives quadratic field scaling, but with a different node sequence: $N_{c,j}\propto(2j+1)B_{c,j}^2$ for a pseudomagnetic field and $N_{c,j}\propto(2j+1)^2B_{c,j}^2$ for energy splitting, where $j$ labels the beating node indices. These results provide quantitative constraints on different microscopic origins of valley- and spin-dependent band splittings in graphene-based systems.