Quantitative analysis of resonant ionization by smooth laser pulses: Connection between effective Hamiltonian theory and strong-field dressed continua

Abstract

Resonant photoionization in the intense high-frequency regime can exhibit extremely asymmetric Autler-Townes doublets whose origin remains debated. It has been attributed either to interference between perturbative ionization pathways or to a non-perturbative dressing of the continuum. Here we show that these interpretations arise from a common effective Hamiltonian framework, in which dressed-state stabilization is governed by the coherent interplay of resonant and nonresonant pathways. We demonstrate that further simplification, using the strong-field approximation, obscures this mechanism. In contrast, our time-dependent essential-state model, where electrons are rigorously coupled to the continuum, achieves excellent agreement with ab initio simulations of the time-dependent Schrödinger equation for helium.