Magnetoresistance in chiral systems driven by inter-band spin-orbit coupling

Abstract

Chiral-induced spin selectivity (CISS), in which electrons transmitted through nonmagnetic chiral materials exhibit strong spin-dependent transport, has attracted growing interest for spintronic applications. However, a quantitative understanding of CISS remains elusive, partly because most previous studies rely on single-band models. In this work, we theoretically investigate multi-band effects on magnetoresistance (MR)-CISS, which is typically observed in experiments using magnetic conductive atomic force microscopy. To evaluate the spin polarization in MR-CISS, we simulate the nonequilibrium steady-state current using the Gorini-Kossakowski-Sudarshan-Lindblad master equation. We find that spin polarization exceeding 25% can be achieved for realistic inter-band spin-orbit coupling strengths in the presence of on-site Coulomb interactions. These findings highlight the crucial role of inter-band spin-orbit coupling in the mechanism of CISS.