Strongly frustrated 2D magnetism in a 3D hexagonal perovskite

Abstract

Exotic quantum phenomena are often found to occur in spin systems that exhibit low-dimensional magnetism. By combining nuclear magnetic resonance, neutron scattering, and muon-spin spectroscopy ($μ$SR) techniques, we report a rare instance of strongly frustrated two-dimensional (2D) magnetism in a three-dimensional (3D) hexagonal perovskite. Here, Ba$_2$La$_2$MnTe$_2$O$_{12}$, a triangular-lattice magnet, is shown to undergo a magnetic transition at $T_\mathrm{N} \approx$ 4.4 K, below which the manganese moments form a 120$^{\circ}$ AFM order within the $ab$-plane, while staying disordered along the $c$-axis. This exotic ground state, which exhibits ideal 2D magnetism, is highly consistent with the persistently strong spin fluctuations and the large internal field distributions revealed by zero-field $μ$SR. Further, the 2D magnetism also leads to a significant frustration, much larger than that of most known magnetically-ordered frustrated systems. Our work on Ba$_2$La$_2$MnTe$_2$O$_{12}$ not only challenges the interpretations of magnetic order in other 3D hexagonal perovskites, but it also provides insight into how the dimensionality affects the exotic magnetic states.