Microscopic origins of inertial magnetization dynamics

Abstract

Ultrafast experiments have uncovered inertial magnetization dynamics in ferromagnets, but their microscopic origin remains elusive. Using a non-Markovian quantum master equation we show that inertial dynamics arise from coherent interactions with optical phonons in the lattice. The fast optical frequency explains the nutation observed on picosecond timescales and accounts for variations between experiments through substrate-dependent phonon damping. By establishing magnon{phonon coupling as the microscopic basis of inertial magnetization, our results open new pathways for tailoring ultrafast spin dynamics and controlling magnetic states at terahertz frequencies.