Electrically tunable interfacial thermal conduction via electronic structure engineering in Au/Bi1-xSbx topological insulators

Abstract

This work provides direct experimental evidence for the role of topological interface states in thermal conduction across a metal/topological insulator junction. It also shows that this conduction can be reversibly modulated by electrical current injection, offering a new approach toward active control of heat flow at solid-state interfaces. Specifically, the interfacial thermal conductance of Au/Bi89Sb11 and Au/Bi87Sb13 junctions demonstrates distinct temperature- and bias-dependent behavior. Both responses are attributed to carrier redistribution between topological interface and bulk band states, driven thermally by Fermi-Dirac broadening and electrically by quasi-Fermi-level shifts and WKB tunneling into nearby bulk bands. Control experiments using trivial semimetals and insulating interlayers further confirm the topological specificity of the effect. Such electrically tunable interfacial heat conduction positions interface electronic structure engineering as a promising route for active thermal management. In doing so, it lays the groundwork for a mechanically robust alternative to conventional structure-driven thermal control compatible with increasingly dense, high-power solid-state devices.

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