Monte Carlo rate uncertainty of the 8Li(n,γ)9Li reaction within R-matrix framework

Abstract

The 8Li(n,γ)9Li reaction is considered significant for the synthesis of nuclei beyond the A=8 stability gap in inhomogeneous big-bang nucleosynthesis models, as well as in r-process nucleosynthesis scenarios. However, direct measurement of this reaction is precluded by the short half-life of 8Li and the absence of a neutron target. Consequently, existing reaction rate estimates based on indirect experimental methods and theoretical calculations differ by orders of magnitude. In the present work, the 8Li(n,γ)9Li neutron-capture cross section and the corresponding thermonuclear reaction rate are evaluated within a phenomenological R-matrix framework, including both non-resonant direct capture (DC) and resonant capture through the 5/2- state at Ex = 4.30~MeV. The uncertainties associated with the R-matrix input parameters are propagated using Monte Carlo sampling, while the sensitivity to the channel radius is treated as an R-matrix model uncertainty. The effective total uncertainties in the calculated cross sections and reaction rates are obtained by adding these two uncertainty contributions in quadrature. We obtain a total capture rate of 983.9+410.9-261.5~cm3\,mol-1\,s-1 at T = 1~GK, with DC dominating at low temperatures (T=0.01-0.4~GK) and the 5/2- resonance at higher temperatures (T=0.5-5~GK). The present results are consistent with the upper limit of Kobayashi et al.~Kobayashi2003, which previous theoretical predictions exceed by factors of 3-50.

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