Correlation-renormalized spin-fluctuation pairing and the stabilization of s superconductivity in pressurized La3Ni2O7
Abstract
The superconducting gap symmetry of pressurized La3Ni2O7 remains unsettled because conventional weak-coupling calculations often place the system close to competing sign-changing s- and d-wave instabilities. Using the four-orbital Wannier Hamiltonian of Xia et al., we combine single-site two-orbital dynamical mean-field theory (DMFT) with a self-energy-renormalized random-phase approximation (RPA). The central step is to replace the bare particle-hole bubble G0G0 of ordinary RPA by a G DMFTG DMFT bubble, while keeping the same residual Slater--Kanamori interaction vertices. In the bare RPA benchmark, the leading pairing eigenvalue belongs to the B2g dxy channel. Once the DMFT self-energy is included, the hierarchy is reversed: the A1g sign-changing s state becomes dominant, the B1g dx2-y2 channel is subleading, and the original B2g instability is strongly suppressed. Pocket-pair decomposition and orbital-resolved susceptibilities show that the reversal originates from orbital-selective renormalization of the d3z2-r2 sector, which filters the γ-pocket scattering processes that stabilize dxy pairing in bare RPA while preserving distributed inter-pocket processes favorable to s pairing. As an independent two-particle validation, we further compute the static spin susceptibility using the dual Bethe--Salpeter equation with the local DMFT vertex. The resulting susceptibility retains a broad finite-momentum magnetic response and is weak near Γ, strengthening the spin-fluctuation background for the correlation-stabilized s state. Our results demonstrate that strong correlations are not a secondary correction in La3Ni2O7: an appropriate treatment of correlation-renormalized quasiparticles is essential for predicting the superconducting pairing symmetry.
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