Emergence of Double-Dome Superconductivity in the Pressurized Dirac Semimetal BaMg2Bi2

Abstract

Dirac semimetal BaMg2Bi2 is reported to be a unique topological material that manifests surface superconductivity that coexistswith bulk band topology at ambient pressure. Here, we present a comprehensive investigation of high-pressure superconductingproperties in BaMg2Bi2 single crystal. Significantly, a pressure-driven double-dome superconducting behavior was revealed, withthe superconducting transition temperature Tc approaching the maximum values of 6.67 K at 4.5 GPa and 7.22 K at 10.4 GPafor the first and second superconducting domes, respectively. The combination of high-pressure X-ray diffraction, Hall resistivitymeasurements, and theoretical calculations demonstrates that, the first superconducting regime is closely related to the pressure-modulated Lifshitz transition, whereas the second superconducting phase emerges concurrently with a structural transition fromthe ambient-pressure P3m1 phase to a high-pressure Pnma phase.