Orbital Correlations in the Ferromagnetic Half-Metal $CrO2

Abstract

We deduce a model relevant for the description of the ferromagnetic half-metal Chromium dioxide (CrO2), widely used in magnetic recording technology. The model describes the effect of dynamical, local orbital correlations arising from local quantum chemistry of the material. A finite temperature solution of the model in d=∞ provides a natural explanation of the optical response, photoemission, resistivity and the large Woods-Saxon ratio observed in experiments. Our study confirms the important role of many body dynamical correlation effects for a proper understanding of the metallic phase of CrO2.

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