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Control of the colossal magnetoresistance by strain effect in Nd0.5Ca0.5MnO3 thin films

E. Rauwel-Buzin, W. Prellier, Ch. Simon, S. Mercone, B. Mercey, B. Raveau, J. Sebek, J. Hejtmanek

cond-mat.mtrl-sciarXiv:cond-mat/0106459

Abstract

Thin films of Nd0.5Ca0.5MnO3 manganites with colossal magnetoresistance (CMR) properties have been synthesized by the Pulsed Laser Deposition technique on (100)-SrTiO3. The lattice parameters of these manganites and correlatively their CMR properties can be controlled by the substrate temperature TS. The maximum CMR effect at 75K, calculated as the ratio ρ(H=0T)/ρ(H=7T) is 104 for a deposition temperature of TS=680 degC. Structural studies show that the Nd0.5Ca0.5MnO3 film is single phase, [010]-oriented and has a pseudocubic symmetry of the perovskite subcell with a=3.77Å at room temperature. We suggest that correlation between lattice parameters, CMR and substrate temperature TS result mainly from substrate-induced strains which can weaken the charge-ordered state at low temperature.

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