Crystal Growth, Transport Properties and Crystal Structure of the Single-Crystal La2-xBaxCuO4 with x=0.11

Abstract

We have attempted the crystal growth by the traveling-solvent floating-zone (TSFZ) method of La2-xBaxCuO4 with x~1/8, where the superconductivity is strongly suppressed. Under flowing O2-gas of a high pressure (4 bars), we have succeeded in growing single crystals of x=0.11 with 5 mm in diameter and 20 mm in length. It has been found that both in-plane and out-of-plane electrical resistivities of the single-crystal La2-xBaxCuO4 with x=0.11 exhibit a clear jump at ~53 K. The temperature corresponds to the structural phase transition temperature between the orthorhombic mid-temperature (OMT) and tetragonal low-temperature (TLT) phases, Td2. It has also been found that both in-plane thermoelectric power and Hall coefficient drop rapidly at Td2 and decrease below Td2 with decreasing temperature. These results are quite similar to those observed in the single-crystal La1.6-xNd0.4SrxCuO4 with x~1/8, suggesting that the so-called static stripe order of holes and spins in the CuO2 plane is formed below Td2 in La2-xBaxCuO4 with x~1/8 as well as in La1.6-xNd0.4SrxCuO4 with x~1/8.

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