Ultrasonic evidence of an uncorrelated cluster formation temperature in manganites with first-order magnetic transition at TC

Abstract

Ultrasonic attenuation and phase velocity measurements have been carried out in the ferromagnetic perovskites La2/3Ca1/3MnO3 and La2/3Sr1/3MnO3. Data show that the transition at the Curie temperature, TC, changes from first- to second-order as Sr replaces Ca in the perovskite. The compound with first-order transition shows also another transition at a temperature T* > TC. We interpret the temperature window TC < T < T* as a region of coexistence of a phase separated regime of metallic and insulating regions, in the line of recent theoretical proposals.

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