Revealing polarons with high pressure on low electron-doped manganites

Abstract

Pressure sensitivity (up to 1 GPa) of the electrical resistivity and of the ac susceptibility was measured for low electron doping levels of Ca1-xYxMnO3 (CYMO) and of Ca1-xSmxMnO3 (CSMO) ceramic samples (0.05 ≤ x ≤ 0.15). A very weak pressure dependence of the Curie temperature (Tc) was observed for both systems ( 6 K GPa-1), when compared to the hole-doped manganites of the same Tc ( 20 K GPa-1). Our results can be interpreted within a modified Double Exchange scenario, where pressure alters the reduction of the bandwidth produced by the electron-phonon interaction associated with small Fr\"ohlich polarons in the weak to intermediate coupling regime.

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