Quasiparticle Relaxation Dynamics in Two Distinct Gap Structures: La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ and LaMnO$_{3}$

Abstract

The spin and quasiparticle relaxation dynamics in La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ and LaMnO$_{3}$ single crystals and thin films is investigated as a function of temperature and magnetic field by pump-probe spectroscopy. The unusually slow spin-lattice relaxation dynamics is governed by the temperature- and magnetic field- dependent pseudogap in La$_{0.67}$Ca$_{0.33}$MnO$_{3}$, and by the temperature-independent Jahn-Teller gap in LaMnO$_{3}$. Our results show that the coupled dynamics of charge, spin and lattice is strongly correlated with the distinct gap structures in these manganites.