Muon Spin Relaxation and Susceptibility Studies of Pure and Doped Spin 1/2 Kagom\'e-like system (CuxZn1-x)3V2O7(OH)2 2H2O

Abstract

Muon spin relaxation (μSR) and magnetic susceptibility measurements have been performed on the pure and diluted spin 1/2 kagom\'e system (CuxZn1-x)3V2O7(OH)2 2H2O. In the pure x=1 system we found a slowing down of Cu spin fluctuations with decreasing temperature towards T 1 K, followed by slow and nearly temperature-independent spin fluctuations persisting down to T = 50 mK, indicative of quantum fluctuations. No indication of static spin freezing was detected in either of the pure (x=1.0) or diluted samples. The observed magnitude of fluctuating fields indicates that the slow spin fluctuations represent an intrinsic property of kagom\'e network rather than impurity spins.

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