Is there a reentrant glass in binary mixtures?
E. Zaccarelli, H. Lowen, P. P. F. Wessels, F. Sciortino, P. Tartaglia, C. N. Likos
Abstract
By employing computer simulations for a model binary mixture, we show that a reentrant glass transition upon adding a second component only occurs if the ratio α of the short-time mobilities between the glass-forming component and the additive is sufficiently small. For α≈ 1, there is no reentrant glass, even if the size asymmetry between the two components is large, in accordance with two-component mode coupling theory. For α 1, on the other hand, the reentrant glass is observed and reproduced only by an effective one-component mode coupling theory.
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