Degenerate perturbation theory of quantum fluctuations in a pyrochlore antiferromagnet

Abstract

We study the effect of quantum fluctuations on the half-polarized magnetization plateau of a pyrochlore antiferromagnet. We argue that an expansion around the easy axis limit is appropriate for discussing the ground state selection amongst the classically degenerate manifold of collinear states with a 3:1 ratio of spins parallel/anti-parallel to the magnetization axis. A general approach to the necessary degenerate perturbation theory is presented, and an effective quantum dimer model within this degenerate manifold is derived for arbitrary spin $s$. We also generalize the existing semiclassical analysis of Hizi and Henley [Phys. Rev. B {\bf 73}, 054403 (2006)] to the easy axis limit, and show that both approaches agree at large $s$. We show that under rather general conditions, the first non-constant terms in the effective Hamiltonian for $s\geq 1$ occur only at {\sl sixth} order in the transverse exchange coupling. For $s\geq 3/2$, the effective Hamiltonian predicts a magnetically ordered state. For $s\leq 1$ more exotic possibilities may be realized, though an analytical solution of the resulting quantum dimer model is not possible.