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Reduction of ordered moment and Neel temperature of quasi one-dimensional antiferromagnets Sr2CuO3 and Ca2CuO3

K. M. Kojima, Y. Fudamoto, M. Larkin, G. M. Luke, J. Merrin, B. Nachumi, Y. J. Uemura, N. Motoyama, H. Eisaki, S. Uchida, K. Yamada, Y. Endoh, S. Hosoya, B. J. Sternlieb, G. Shirane

cond-mat.str-elarXiv:cond-mat/9701091

Abstract

We report elastic neutron diffraction and muon spin relaxation (muSR) measurements of the quasi one-dimensional antiferromagnets Sr2CuO3 and Ca2CuO3, which have extraordinarily reduced TN/J ratios. We observe almost resolution-limited antiferromagnetic Bragg reflections in Sr2CuO3 and obtain a reduced ordered moment size of ~0.06 μB. We find that the ratio of ordered moment size μ(Ca2CuO3)/μ(Sr2CuO3)=1.5(1) roughly scales with their Neel temperatures, which suggests that the ordered moment size of quasi one-dimensional antiferromagnets decreases continuously in the limit of vanishing inter-chain interactions.

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