Observation of Spin Freezing in CaV4O9 and CaV2O5 by uSR
Abstract
We have performed muon spin relaxation and susceptibility measurements of CaV4O9 and CaV2O5, systems in which spin gap-like behavior has been found. We observe spin freezing in the two compounds below 12K and 50K, respectively. Our results indicate the possibility that a substantial fraction of the of the vanadium magnetic moment is not in a spin singlet sate at low temperatures in either material.
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