Manganites at Low Temperatures and Light Doping:Band Approach and Percolation

Abstract

A tight-band model is employed for the e2g-orbitals in manganites. It is shown that a large intraatomic Hund's coupling, JH and the resulting double-exchange mechanism lead to antiferromagnetic ordering along one of the cubic axis stabilized by the cooperative JT effect which further decreases the band energy of electrons. As a result, LaMnO3 is a band insulator built of 2D ferromagnetic layers. The critical concentration xc 0.16, for onset of ferromagnetic and metallic behavior at low temperatures in La1-xSrxMnO3 and the phase transition are treated in the percolation approach.

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