Theory of Ferromagnetic Metal to Paramagnetic Insulator Transition i in R1-xAxMnO3

Abstract

The double-exchange model for the Mn oxides with orbital degeneracy is studied with including on-site Coulomb repulsion, Jahn-Teller (J-T) coupling and doping-induced disorder. In the strong interaction limit, it is mapped onto a single-band Anderson model, in which all scattering mechanisms can be treated on an equal footing. A sharp rise in the mean square fluctuation of lattice distortions is found near the Curie temperature Tc, in agreement with experiments. We show that the spin and J-T disorders lead to a metal-insulator transition (MIT) only at low carrier density. The MIT observed in samples with 0.2≤ x<0.5 can be explained by further including the disorder effect of cation size mismatch.

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