Frequency modulation and pulse compression by coherent multimode molecular motion

Abstract

We study beating of a probe field with a time-varying susceptibility in a coherently prepared Raman medium. We consider the general case of an arbitrary variation of susceptibility, which corresponds to a superposition of an arbitrary number of excited Raman transitions. We derive a general analytical solution and conservation relations for this process. We show that the interference between Raman polarizations may substantially affect frequency modulation and pulse compression for the probe field.