Production and chemical separation of $^{229}$Pa toward observation of ${\gamma}$ rays of $^{229\rm{m}}$Th

Abstract

To observe the ${\gamma}$ rays emitted from the low-lying isomeric state of $^{229}$Th ($^{229\rm{m}}$Th), we aim to dope fluoride crystals with its precursor $^{229}$Pa. In this study, we produced $^{229}$Pa by a 30-MeV proton bombardment on $^{232}$Th and developed a chemical separation method. The chemical yield of Pa was 93(4)%, and the physical production yield of $^{229}$Pa for the proton energy range of 29.0${-}$30.1 MeV was measured to be 9.4(8) MBq/${\rm{\mu}}$Ah, which was more than 10 times higher than those of $^{232,230,228,233}$Pa. These high chemical and production yields will allow us to prepare fluoride crystals having a sufficient amount of $^{229}$Pa for the observation of the ${\gamma}$ rays of $^{229\rm{m}}$Th.