Attosecond delay metrology beyond the photon coherence time with spectrally resolved Hong-Ou-Mandel interferometry

Abstract

Hong-Ou-Mandel (HOM) interferometry enables delay estimation at the quantum precision limit but is traditionally constrained to path differences within the coherence time of the interfering photons. Here, we demonstrate single-measurement path-delay sensing at the measurement Cramer-Rao bound using spectrally resolved HOM interference, thereby removing the conventional dynamic-range limitation imposed by the photon coherence window, with no scanning required for calibration. By extracting delay information from the spectral interference fringes of spectrally entangled photon pairs, we retain near-optimal sensitivity over an operational range exceeding the photon coherence time by over two orders of magnitude. Using one million detected photon pairs, we achieve a time-delay precision of 20 attosecond (6 nm), while real-time operation (at 1 Hz) yields 330 attosecond (100 nm) precision. Because the estimator relies on fringe periodicity rather than absolute coincidence rates, the method is intrinsically robust to photon losses and variations in interference visibility, eliminating the need for recalibration. As a practical demonstration, we measure the thickness of a 300 um transmissive target with nanometer-scale precision. These results mark a significant step towards deploying quantum-limited measurements in real-world sensing applications using HOM interferometry.